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Creators/Authors contains: "Fullerton, Eric_E"

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  1. Abstract Manipulating the topological properties of spin textures in magnetic materials is of great interest due to the rich physics and promising technological applications of these materials in advanced electronic devices. A spin texture with desired topological properties can be created by magnetic monopole injection, resulting in topological transitions involving changes in the topological charge. Therefore, controlling magnetic monopole injection has paramount importance for obtaining the desired spin textures but has not yet been reported. Here, we report the use of reliably manipulated magnetic monopole injection in the topological transition from stripe domains to skyrmions in an Fe/Gd multilayer. An easily tunable in-plane magnetic field applied to an Fe/Gd multilayer plays a key role in the magnetic monopole injection by modulating the local exchange energy. Our findings facilitate the efficient management of topological transitions by providing an important method for controlling magnetic monopole injection. 
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  2. Abstract Herein, the experimental observation of micrometer‐scale magnetic skyrmions at room temperature in several Pt/Co‐based thin film heterostructures designed to possess low exchange stiffness, perpendicular magnetic anisotropy, and a modest interfacial Dzyaloshinskii–Moriya interaction (iDMI) is reported. It is found both experimentally and by micromagnetic and analytic modeling that a low exchange stiffness and modest iDMI eliminates the energetic penalty associated with forming domain walls in thin films. When the domain wall energy density approaches negative values, the remanent morphology transitions from a uniform state to labyrinthine stripes. A low exchange stiffness, indicated by a sub‐400 K Curie temperature, is achieved in Pt/Co, Pt/Co/Ni, and Pt/Co/Ni/Re structures by reducing the Co thickness to the ultrathin limit (<0.3 nm). Similar effects occur in thicker Pt/Co/NixCu1−xstructures when the Ni layer is alloyed with Cu. At this transition in domain morphology, skyrmion phases are stabilized by small (<1 mT), perpendicular magnetic fields, and skyrmion motion in response to spin–orbit torque is observed. While the temperature and thickness‐induced morphological phase transitions observed are similar to the well‐studied spin reorientation transition that occurs in the ultrathin limit, the underlying energy balances are substantially modified by the presence of an iDMI. 
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  3. Abstract Magnetic skyrmions exhibit unique, technologically relevant pseudo‐particle behaviors which arise from their topological protection, including well‐defined, 3D dynamic modes that occur at microwave frequencies. During dynamic excitation, spin waves are ejected into the interstitial regions between skyrmions, creating the magnetic equivalent of a turbulent sea. However, since the spin waves in these systems have a well‐defined length scale, and the skyrmions are on an ordered lattice, ordered structures from spin‐wave interference can precipitate from the chaos. This work uses small‐angle neutron scattering (SANS) to capture the dynamics in hybrid skyrmions and investigate the spin‐wave structure. Performing simultaneous ferromagnetic resonance and SANS, the diffraction pattern shows a large increase in low‐angle scattering intensity, which is present only in the resonance condition. This scattering pattern is best fit using a mass fractal model, which suggests the spin waves form a long‐range fractal network. The fractal structure is constructed of fundamental units with a size that encodes the spin‐wave emissions and are constrained by the skyrmion lattice. These results offer critical insights into the nanoscale dynamics of skyrmions, identify a new dynamic spin‐wave fractal structure, and demonstrate SANS as a unique tool to probe high‐speed dynamics. 
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  4. Abstract All‐optical control and detection of magnetic states for high‐density recording necessitate nanophotonic approaches to amplify local light intensity below the diffraction limit. Sculpting the near‐field phase and polarization can additionally strengthen magneto‐optical effects that rely on circularly polarized pulses, such as all‐optical helicity‐dependent switching, imaging, and spin‐wave excitation. Here, high‐refractive‐index dielectric nanoantennas illuminated with circularly polarized light resonantly enhance local electric field rotation by more than sixfold within [Pt/Co]Nthin films. Sub‐wavelength arrays of amorphous Si nanodisks, or metasurfaces, patterned on perpendicularly magnetized films support Mie‐type resonances that modulate reflection and transmission dissymmetry by >±2% in experiments. Spatial and spectral interference between dipolar modes, proximity effects, and gain are evaluated by varying disk aspect ratio, metasurface–metal separation, and magnetic film thickness, respectively. Simulated enhancements in magnetic circular birefringence and differential absorption are correlated with amplified local field rotation at electric dipolar modes. Greater achievable amplifications are shown via simulations with single‐crystalline Si metasurfaces exhibiting lower losses, including a 12‐fold strengthened electric field rotation within ferromagnetic layers. The metasurface design rules established here could enable nanoscale localization of all‐optical magnetic switching with lowered laser fluence thresholds, as well as enhanced magneto‐optical responses for light‐assisted reading in spintronic devices. 
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